The C entry for the limiting reactant must be the negative of the starting amount, since it is all used up in the reaction.
The C entries for the other reactants and products are related to the limiting reactant by stoichiometric factors. For example, the C entry for NO (g) is as large as the C entry of the limiting reactant. It has a positive sign since its amount is increasing.
The E entries are found by adding together the I and C entries for each column.