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B.S., 1993, Seoul National University
M.S. 1995, Seoul National University
Ph.D., 2000, Michigan State University
Postdoctoral Research Associate at University of California, Santa Barbara, 2000-2002
Our research focuses on design, synthesis, and characterization of semiconducting and metallic crystals and thin film-type electrodes with controlled micro- and nano-structures for use in electrochemical and photoelectrochemical devices (e.g. photoelectrochemical cells, fuel cells, and rechargeable batteries, and sensors). This research combines disciplines of inorganic chemistry, solid state chemistry, electrochemistry, materials chemistry, and nano-scale science.
When electrochemical and photoelectrochemical devices contain polycrystalline electrodes or catalysts, variances of particle shapes, sizes, orientations, and interconnections significantly affect the chemical and physical factors that define the energetics and kinetics of these electrodes or catalysts. Therefore, controlling and understanding the effects of micro- and nano-structural features at the interface on functional properties are the keys to producing highly efficient, cost effective, and lightweight devices.
In order to accomplish these tasks our group develops new electrochemical synthetic strategies that can make a significant advancement in constructing polycrystalline electrode materials. We achieve this by combining compositionally versatile electrodeposition methods with various new synthetic concepts/techniques that can allow for precise morphological control at various length scales (e.g. electrochemical interfacial supramolecular templating, controlled electrocrystallization). Since electrodeposition is based on a low-temperature solution-based method with many synthetic variables that can be precisely and freely controlled, our approach allows for the assembly of a broad range of inorganic electrodes with systematically varying micro- and nano-structural features (e.g. mesoporous films, nano- and micro-scale crystal engineering).
The functional properties we currently investigate in conjunction with morphological variation include optical, electrochemical, photoelectrochemical, and photo-/electro-catalytic properties. By pursuing an in-depth atomic level understanding of structure-property relationships as well as efficiency enhancement by interfacial engineering, we attempt to bridge the gap between chemistry and materials engineering.
Awards and Honors
|University of Wisconsin-Madison Vilas Associate Award||2016|
|Wisconsin Alumni Research Foundation Innovation Award||2015|
|Camille and Henry Dreyfus Environmental Chemistry Mentor||2015|
|Speaker, Stanford Distinguished Women in Science Colloquium||2014|
|Outstanding Undergraduate Teaching Award by an Assistant Professor, Purdue College of Science||2008|
|Combined Experimental and Theoretical Investigations of n-Type BiFeO3 for Use as a Photoanode in a Photoelectrochemical Cell. Chemistry of Materials. 2020;32:3262-3270..|
|The Role of Surface Oxygen Vacancies in BiVO4. Chemistry of Materials. 2020;32:2899-2909..|
|Impacts of the Regeneration Pathways of the Oxoammonium Cation on Electrochemical Nitroxyl Radical-Mediated Alcohol Oxidation. ACS Catalysis. 2020;10:265-275..|
|Photoelectrochemical Nitrogen Reduction to Ammonia on Cupric and Cuprous Oxide Photocathodes. ACS Energy Letters. 2020;:1834-1839..|
|A Comparative Study of Nickel, Cobalt, and Iron Oxyhydroxide Anodes for the Electrochemical Oxidation of 5-Hydroxymethylfurfural to 2,5-Furandicarboxylic Acid. ACS Catalysis. 2019;9:660-670..|